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What really drives electron spin decoherence in molecular crystals at low-T? Nuclear or Electron spins? Turns out you have do magnetically dilute your samples quite a bit if you want to really remove electron-electron dipolar interactions... pubs.aip.org/aip/jcp/arti...
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The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectrosc
Spin decoherence in molecular crystals: Nuclear vs electronic spin baths
pubs.aip.org
Alessandro Lunghi